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Abstract In this work, we explore how the optical properties of isotropic materials can be modulated by adjacent anisotropic materials, providing new insights into anisotropic light-matter interactions in van der Waals heterostructures. Using a WS₂/ReS₂heterostructure, we systematically investigated the excitation angle-dependent photoluminescence (PL), differential reflectance, time-resolved PL, and power-dependent PL anisotropy of WS₂. Our findings reveal that the anisotropic optical response of WS₂, influenced by the crystallographically low symmetry and unique dielectric environment of ReS₂, significantly impacts both the optical and temporal behavior of WS₂. We observed that the emission anisotropy increases with optical power density, highlighting that anisotropic localization of photo-generated carriers and subsequent charge transfer dynamics are key contributors to the polarization-sensitive optical response. These findings provide a framework for leveraging optical density-sensitive anisotropy mirroring to design advanced anisotropic optoelectronic and photonic devices.